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- W2017463670 abstract "Both photochemical and nonphotochemical spectral hole burning mechanisms were observed in the incommensurate phase III (ICIII) of chlorin-doped biphenyl. Distributions of corresponding energetic barriers for the back reaction were acquired from temperature cycling experiments. The non-photochemical mechanism is characterized by finite (unlike to glasses) but low (compared to the photochemical mechanism) threshold of 6--7 K and is interpreted as a photoinduced depinning-repinning of the incommensurate modulation wave. Holewidth dependence on cycling temperature up to 28 K was measured, crossing at 17 K the phase transition between two incommensurate phases in pure biphenyl. The measured irreversible hole broadening exhibits a fast (close to cubic) increase up to 17 K and then changes abruptly to a linear in the higher-temperature incommensurate phase II, which extrapolates back to zero at $stackrel{ensuremath{rightarrow}}{T}0mathrm{K}.$ The results support the view that ICIII is a metastable state." @default.
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- W2017463670 date "2001-08-23" @default.
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- W2017463670 title "Irreversible dynamics in incommensurate biphenyl studied by thermocycling of spectral holes" @default.
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- W2017463670 doi "https://doi.org/10.1103/physrevb.64.104203" @default.
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