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- W2017535245 abstract "A molecular-confinement model is proposed for the calculation of density effects on the electronic stopping cross section ${(S}_{e})$ in a condensed medium. In this model, the collective intermolecular interactions in the medium are represented by a mean field in which a particular molecule is embedded including the spatial constrictions imposed by the surrounding molecules. A molecule is thus viewed as a caged-in system within a spherical boundary with finite potential barrier height ${V}_{B}.$ Changes in the molecular electronic properties and molecular conformation as a function of medium density are self-consistently treated. As a first example of a general treatment for more complicated target structures, the model is explicitly applied to the case of proton stopping in dense molecular hydrogen. The lowest barrier height ${(V}_{B}=0)$ was selected for the stopping calculations since it provides a more realistic pressure-density relation at $T=0mathrm{K}$ than higher barrier values. Our results for dense molecular hydrogen predict a very small to moderate reduction in ${S}_{e}$ relative to the gas phase in going from atmospheric pressure (0.036 ${mathrm{m}mathrm{o}mathrm{l}/mathrm{c}mathrm{m}}^{3}$, $ensuremath{Delta}{S}_{e}ensuremath{approx}0.5%$) up to 136 GPa (0.380 ${mathrm{m}mathrm{o}mathrm{l}/mathrm{c}mathrm{m}}^{3}$, $ensuremath{Delta}{S}_{e}ensuremath{approx}24%$) for either the liquid or solid phase as determined by the phase diagram for this medium." @default.
- W2017535245 created "2016-06-24" @default.
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- W2017535245 date "1999-09-01" @default.
- W2017535245 modified "2023-10-18" @default.
- W2017535245 title "Proton stopping in dense molecular hydrogen: A molecular-confinement model" @default.
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- W2017535245 doi "https://doi.org/10.1103/physreva.60.2207" @default.
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