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- W2017609815 abstract "In this work, the sequence of two elementary processes called dehydrodimerization, namely (i) RH+M.→R.+HM and (ii) 2R.→RR are considered. These reactions are particularly helpful for cleaning a medium from free radicals (radioprotection of the medium). In the first step the trapping of radical M. generates a hydrogenated product MH and another radical R. which disappears in the second step. Both abstraction and recombination reactions obey an Evans—Polanyi type of relation: the activation energies linearly depend on the dissociation energies of the bond (s) involved in the corresponding process. In this paper, a theoretical approach to the classification of RH compounds according to their capability to behave as good radical scavengers is proposed. It is shown that good candidates should have a small BDE (RH) and correspond to RR dimers having either very small or rather large BDE(RR)." @default.
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- W2017609815 date "1988-10-01" @default.
- W2017609815 modified "2023-09-27" @default.
- W2017609815 title "A theoretical approach to dehydrodimerization reactions" @default.
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- W2017609815 doi "https://doi.org/10.1016/0166-1280(88)80126-x" @default.
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