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• W2017926503 abstract "Half-titanocenes containing aryloxide ligands immobilized on the chain end of ring-opened poly(norbornene)s, (C5Me5)TiMe2[O-2,6-R2C6H2-4-CH{CH-(1,3-cyclo-C5H8)-CH}nCHCMe2Ph] [R = H (1), Me (2), iPr (3)], prepared by living ring-opening metathesis polymerization (ROMP) by Mo(N-2,6-iPr2C6H3)(CHCMe2Ph)(OtBu)2, have been prepared and identified by 1H and 13C NMR spectra, elemental analysis, and X-ray photoelectron spectroscopy. These complexes showed high catalytic activities for ethylene polymerization in the presence of methylaluminoxane (MAO) cocatalyst, and the effect of the substituent on the aryloxide on both the activity and molecular weight of the resultant polymer was the same as that using nonsupported (C5Me5)TiCl2(O-2,6-R2C6H3) (R = H, Me, iPr). Complex 3 showed both notable catalytic activities and efficient 1-hexene incorporation with the same monomer reactivity ratio as nonsupported (C5Me5)TiCl2(O-2,6-iPr2C6H3) (3‘) for ethylene/1-hexene copolymerization in the presence of MAO." @default.
• W2017926503 created "2016-06-24" @default.
• W2017926503 creator A5048382701 @default.
• W2017926503 creator A5090798467 @default.
• W2017926503 date "2007-06-08" @default.
• W2017926503 modified "2023-10-11" @default.
• W2017926503 title "Synthesis of Half-Titanocenes Containing Aryloxide Ligands Attached to the ROMP Polymer Chain End: Unique Catalyst Precursors for Ethylene (Co)polymerization" @default.
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• W2017926503 doi "https://doi.org/10.1021/om0701064" @default.
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