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• W2018013067 abstract "Abstract Detection of atoms by mass spectrometry has been used to study the reactions of hydrogen azide, HN 3 , with H atoms and active nitrogen, in a fast flow reactor at pressures of about 1 torr. Stoichiometry and products of the H + HN 3 reaction have been determined and the rate constant of the initial step, assumed to be H + HN 3 → NH 2 + N 2 , was found to be 2.54 × 10 −11 exp (−4600/ RT ) cm 3 molecule −1 s −1 , in the temperature range of 300–460K. The formation of NH 3 and H 2 products has been discussed from the different secondary steps which may occur in the mechanism. For the reaction of active nitrogen with HN 3 , evidence has been found for the participation of excited nitrogen molecules produced by a microwave discharge through molecular nitrogen. The influence of excited nitrogen molecules has been reduced by lowering the gas flow velocity. It was then possible to study the N + HN 3 reaction for which the rate constant of the initial step was found to be 4.9 × 10 −15 cm 3 molecule −1 s −1 at room temperature. Finally, the occurrence of these elementary reactions has been discussed in the mechanism of the decomposition flame of HN 3 ." @default.
• W2018013067 created "2016-06-24" @default.
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• W2018013067 creator A5076584938 @default.
• W2018013067 date "1973-07-01" @default.
• W2018013067 modified "2023-10-10" @default.
• W2018013067 title "The reactions of atomic hydrogen and active nitrogen with hydrogen azide" @default.
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• W2018013067 doi "https://doi.org/10.1002/kin.550050407" @default.
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