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- W2018024022 abstract "We present L2,3 X-ray emission spectra of the 3d-metals Ti through Cu. It is found that the ratio of the integrated non-resonant emission intensities of L2 to L3 emission, I(L2)/I(L3), is approximately two times smaller than the ratio of the core hole state degeneracies (L2/L3 = 1/2). Our atomic calculations show that the L2L3M4,5 Coster–Kronig transition is responsible for the reduction of the I(L2)/I(L3) intensity ratio and explains its gradual decrease with increasing atomic number among the 3d transition metals. For the resonant case we find that accounting for the core–hole interaction and local field effects via TDDFT satisfactorily explains the changes in the I(L2)/I(L3) ratio." @default.
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- W2018024022 date "2005-07-01" @default.
- W2018024022 modified "2023-09-23" @default.
- W2018024022 title "The L2:L3 intensity ratio in soft X-ray emission spectra of 3d-metals" @default.
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- W2018024022 doi "https://doi.org/10.1016/j.elspec.2005.01.266" @default.
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