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• W2018115546 abstract "Polycyclic structures that contain seven-membered carbocycles constitute important structural motifs that are ubiquitous in several classes of bioactive natural products. We have developed the first regio- and diastereoselective intermolecular rhodium-catalyzed [3+2+2] carbocyclization of carbon- and heteroatom-tethered alkenylidenecyclopropanes with mono- and disubstituted alkynes for the construction of cis-fused bicycloheptadienes. This study delineates some of the critical features for controlling regioselectivity in this process and demonstrates that E-alkenes can be incorporated in a stereospecific manner to afford products with up to three new stereogenic centers. The latter feature is particularly significant given that related carbocyclization reactions are often limited in this respect." @default.
• W2018115546 created "2016-06-24" @default.
• W2018115546 creator A5036451127 @default.
• W2018115546 creator A5080435243 @default.
• W2018115546 date "2008-09-09" @default.
• W2018115546 modified "2023-10-10" @default.
• W2018115546 title "Intermolecular Rhodium-Catalyzed [3+2+2] Carbocyclization of Alkenylidenecyclopropanes with Activated Alkynes: Regio- and Diastereoselective Construction of <i>cis</i>-Fused Bicycloheptadienes" @default.
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• W2018115546 doi "https://doi.org/10.1021/ja803691p" @default.
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