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• W2018150012 abstract "A complete set of electron-excited 4d-basedAuger spectra of the lanthanide metals from lanthanum to lutetium (except the unstable promethium) is presented, in both differential and integral forms. It is believed that the set is more representative of clean surfaces of the lanthanides than any published hitherto. With the help of binding energy and electron loss measurements made in this laboratory and elsewhere, values of the various possible Auger, Coster—Kronig, and direct recombination transition energies are calculated, and for each transition a “centre of gravity” is derived based on relative intensities of final state multiplets, electron occupation of core levels, etc. By using arguments based on trends in the spectra across the series, on theoretically and experimentally derived values of Ueff for the difference 4fn+1→4fn−1, and on plausibility, values of Ueff for 4fn→ 4fn−2 as well as for the other final state hole pair configurations are allocated. The relaxed transition energies so calculated are then compared with the experimental energies, from which it is possible in most cases to make assignment of the spectral features to the various transitions. As a result it is found that there are some significant disagreements with the theoretical rates of McGuire for lanthanide free atoms. The reasons for these disagreements are discussed, and an empirical model based on effective 4f and 5d populations and on the restrictions imposed by spin alignment is used to resolve the differences qualitatively." @default.
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• W2018150012 date "1985-01-01" @default.
• W2018150012 modified "2023-10-17" @default.
• W2018150012 title "The 4d auger, coster-kronig, and recombination spectra of the lanthanides" @default.
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• W2018150012 doi "https://doi.org/10.1016/0368-2048(85)80030-x" @default.
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