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- W2018172005 abstract "Abstract The oxidation of a mixed uranium dicarbide and graphite powder has been investigated by simultaneous thermal gravimetric (TGA) and differential thermal (DTA) analyses coupled with gas phase chromatography. For isothermal oxidation conditions with temperatures below 330 °C, only the UC 2 chemical phase is progressively oxidised into U 3 O 8 oxides. Parabolic weight gain curves as a function of oxidation over time were obtained. A detailed kinetic study is proposed to establish a pseudo-steady-state during the oxidation process. Using an experimental method based on the sudden temperature increases, a single rate-limiting step has been validated and then modelled by a 3D diffusion law. An apparent activation energy calculated from the Arrhenius representation has been evaluated at −35 kJ/mol, thus describing the diffusion of oxygen through the oxide layer." @default.
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- W2018172005 date "2013-06-01" @default.
- W2018172005 modified "2023-09-23" @default.
- W2018172005 title "Oxidation kinetic analysis of a mixed uranium dicarbide and graphite compound" @default.
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- W2018172005 doi "https://doi.org/10.1016/j.jnucmat.2013.02.028" @default.
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