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• W2018203957 endingPage "769" @default.
• W2018203957 startingPage "763" @default.
• W2018203957 abstract "A method using CO2 and PhSiH3 for the methylation of primary and secondary aliphatic amines catalyzed by Ni (0) complexes was developed, selectively producing the monomethylated products in moderate to good yields. For that purpose, two catalysts were used: [(dippe)Ni(μ-H)]2 and the commercially available Ni(COD)2/dcype, both of which were rather efficient in this process. With a slight experimental modification, the reaction allowed the production of monomethylated ureas in good yields by using low amounts of PhSiH3. On the basis of the experimental results, we propose a possible reaction mechanism for the formation of the new C–N bond." @default.
• W2018203957 created "2016-06-24" @default.
• W2018203957 creator A5047892519 @default.
• W2018203957 creator A5065768436 @default.
• W2018203957 creator A5086702064 @default.
• W2018203957 date "2015-01-30" @default.
• W2018203957 modified "2023-10-18" @default.
• W2018203957 title "Selective <i>N</i>-Methylation of Aliphatic Amines with CO₂ and Hydrosilanes Using Nickel-Phosphine Catalysts" @default.
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• W2018203957 doi "https://doi.org/10.1021/om501176u" @default.
• W2018203957 hasPublicationYear "2015" @default.
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