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- W2018261852 abstract "Abstract Summary: We study the impact of topological disorder on the mechanical response of hyperbranched macromolecules from a theoretical and numerical perspective. The polymer models are generated using a bond switching algorithm, and the emerging systems are described within the Zimm and Rouse pictures of macromolecular dynamics. The topological disorder is manifest in the frequency‐dependent dynamic moduli, $G^*(omega)$ . These are clearly distinct from that of regular hyperbranched fractals of the same size, and they do not obey simple scaling rules. The dynamic moduli reflect the short‐range order inherent in the model, and we thus suggest that the extent of disorder in branched tree‐like polymers may be well‐estimated experimentally using $G^*(omega)$ . Model of an irregular hyperbranched polymer. magnified image Model of an irregular hyperbranched polymer." @default.
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- W2018261852 date "2006-08-15" @default.
- W2018261852 modified "2023-10-10" @default.
- W2018261852 title "Models of Irregular Hyperbranched Polymers: Topological Disorder and Mechanical Response" @default.
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- W2018261852 doi "https://doi.org/10.1002/mats.200600004" @default.
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