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• W2018363439 abstract "Abstract For emulsion polymerization of a ‘zero-one’ system, the method of moments is applied to the model proposed by Lichti et al. to describe the particle size distribution (PSD). Using the explicit expressions so obtained for the first four moments, the average number of free radicals par particle, n ss , and kinetic parameters of the system involving the rate coefficients for adsorption and desorption of free radicals, ϱ and κ, and the propagation rate coefficient, κp, can be obtained easily by use of PSD data without involving a complicated curve fitting procedure as was required in their work. Detailed calculations on the styrene system data of Lichti et al. show that both ϱ and κ are proportional to particle surface area. The result for κ is opposite to that proposed by those workers, in which κ was considered to be inversely proportional to the particle surface area. After further manipulation and approximation of the expressions so obtained, explicit expressions for the number-average volume, gn n , the standard deviation, σ, and the skewness, u′3, in terms of surfactant and initiator levels, temperature and reaction time are also obtained. The effects of the variations of these variables on the three characteristic parameters of the PSD can be determined." @default.
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• W2018363439 date "1988-03-01" @default.
• W2018363439 modified "2023-10-11" @default.
• W2018363439 title "Emulsion polymerization: determinations of the average number of free radicals per particle and kinetic parameters by use of the particle size distribution" @default.
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• W2018363439 doi "https://doi.org/10.1016/0032-3861(88)90376-x" @default.
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