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- W2018377208 abstract "The stochastic Liouville equation is used to discuss the role of fluctuations in tunneling dynamics. Emphasis is given to the case where the matrix elements of the hamiltonian are continuous-time Markov chains, since in this case the computational scheme is shown to be very simple, being based on matrix manipulations. The utility of the method for arbitrary correlation times is illustrated in two examples concerning two-level proton tunneling. In the first the role of a fluctuating electric field created by the solvent is discussed and the results are interpreted in terms of “motional narrowing”. In the second example the influence of a strong electromagnetic field (which determines jumps between two potential energy curves) is analyzed for a concrete case, i.e. the tropolone molecule." @default.
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- W2018377208 date "1987-08-01" @default.
- W2018377208 modified "2023-09-25" @default.
- W2018377208 title "Tunneling in the presence of fluctuations: the stochastic liouville equation approach" @default.
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- W2018377208 doi "https://doi.org/10.1016/0301-0104(87)80051-4" @default.
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