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- W2018446578 abstract "Four most prominent features of the volume recovery in glasses of different nature, including polymeric ones, such as non-linearity, asymmetry, memory effects and hysteresis phenomena are analyzed on the basis of a simple diffusion model. The kinetics of the structural recovery is assumed to be controlled by the diffusion of free volume in a sample. Thus, the above mentioned effects are referred to specific evolution of the spatial distribution (profile) of the free volume. Apart from this, the dependence of diffusion coefficient D on the free volume fraction f is introduced for the correct description of the experiments. Computer simulations of the corresponding experiments have been performed using functions D (f) of different types: D = A·exp (-B/f), D = A·exp (B.f) and D = A·fn. The curves of the volume recovery and the corresponding profiles of the free volume in samples have been obtained as a result of computation. All these results are shown to coincide quantitatively with the available literature data on the volume recovery and to be practically independent of the choice of D (f) function type." @default.
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- W2018446578 date "1984-03-01" @default.
- W2018446578 modified "2023-09-27" @default.
- W2018446578 title "Diffusion model of volume recovery in glasses" @default.
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- W2018446578 doi "https://doi.org/10.1002/macp.1984.020061984123" @default.
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