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• W2018472223 abstract "We study a model of heterogeneous catalysis with competitive reactions between two monomers A and B. We assume that reactions are dependent on temperature and follow an anti-Arrhenius mechanism. In this model, a monomer A can react with a nearest neighbor monomer A or B, however, reactions between monomers of type B are not allowed. We assume attractive interactions between nearest neighbor monomers as well as between monomers and the catalyst. Through mean-field calculations, at the level of site and pair approximations, and extensive Monte Carlo simulations, we determine the phase diagram of the model in the plane yA versus temperature, where yA is the probability that a monomer A reaches the catalyst. The model exhibits absorbing and active phases separated by lines of continuous phase transitions. We calculate the static, dynamic, and spreading exponents of the model, and despite the absorbing state be represented by many different microscopic configurations, the model belongs to the directed percolation universality class in two dimensions. Both reaction mechanisms, Arrhenius and anti-Arrhenius, give the same set of critical exponents and do not change the nature of the universality class of the catalytic models." @default.
• W2018472223 created "2016-06-24" @default.
• W2018472223 creator A5004781150 @default.
• W2018472223 creator A5044726409 @default.
• W2018472223 date "2012-04-23" @default.
• W2018472223 modified "2023-10-16" @default.
• W2018472223 title "Absorbing states in a catalysis model with anti-Arrhenius behavior" @default.
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• W2018472223 doi "https://doi.org/10.1063/1.4705361" @default.
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• W2018472223 hasPublicationYear "2012" @default.
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