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- W2018502592 abstract "Without actually evaluating the integrals involved, an experimental technique and a mode of analysis have been developed to quantitatively verify van Vleck’s theory of vibronic interactions. The success of the analysis suggests that errors introduced by the computational approximations far outweight those introduced by the partial breakdown of the assumptions upon which the theory is constructed. Specifically, the vibronic transition at 21 200 cm -1 of Co(NH 3 )6 3+ has been used to discuss the techniques developed. Furthermore, it has been established that at all temperatures from 293 °K down to 83 °K the ν̃ 6 vibrational mode of the MX 6 entity is primarily responsible (60%) for the admixture of odd parity in the ground and the first excited states of Co (NH 3 ) 6 3+ ." @default.
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- W2018502592 date "1969-02-01" @default.
- W2018502592 modified "2023-09-23" @default.
- W2018502592 title "Relative Contributions of Odd Vibrations to the Intensity of the First Band of Co(NH<sub>3</sub>)6<sup>3+</sup>" @default.
- W2018502592 doi "https://doi.org/10.1515/zna-1969-0211" @default.
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