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- W2018618692 abstract "Studies of relaxation in rubbery networks reveal a variety of behaviours. In experiments on networks with labelled junctions, whereby the motion of the crosslink site is specifically monitored, the segmental relaxation function broadens with increasing crosslink density, accompanied by a larger activation energy. Such results are well-described by theory. The more usual experiment simply measures bulk relaxation, without discriminating among different relaxing entities. For networks, crosslinking introduces a distribution of relaxation behaviours, related to the proximity of a moiety to the junctions. The resulting inhomogeneously broadened relaxation function is difficult to analyse; nevertheless, a heightened sensitivity to temperature (larger activation energy) is observed, from which inferences can be made regarding the shape of the segmental relaxation function. Crosslinking also influences the viscoelastic spectrum at times longer than that associated with local segmental relaxation, in a manner consistent with ideas based on constraint dynamics." @default.
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- W2018618692 date "1997-01-01" @default.
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- W2018618692 title "The viscoelastic behaviour of networks" @default.
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