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- W2018684472 abstract "We propose that the unusual frequency dependent lineshapes observed in Raman scattering experiments on polyacetylene are due to hot luminescence in very long polyene chains. Employing a generalized equation of motion technique we find that a photoexcited polyene is unstable with respect to a variety of symmetry lowering distortions which vary as a function of the frequency of the exciting radiation. Radiative decay during this relaxation is observably strong in the inelastically scattered photon spectrum and would explain the dominant observed lineshape variations." @default.
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- W2018684472 title "Hot luminescence in polyacetylene" @default.
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- W2018684472 doi "https://doi.org/10.1016/0038-1098(82)90283-6" @default.
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