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- W2018721935 abstract "The rates of formation of hydrates of H3O+ in the reactions H3O+(H2O)n−1+H2O+M⇆H3O+(H2O)n+M, n = 1, 2, 3, were studied using drift tube techniques. Experiments were performed at 337°K with mixtures of 0.5% to 1.8% partial pressure of water in argon at total pressures from 0.6 to 3.0 torr. Rate constants for the forward reactions decreased slowly with increasing E / P0 in the range 4–30 V cm−1·torr−1. Values for k1, k2, and k3 at 337°K were 6 × 10−28, 6 × 10−28, and 2 × 10−28 cm6/sec. Limits were estimated for the reverse reactions. Mobilities of the cluster sequence from H3O+ to H9O4+ were almost independent of E / P in the range studied, with zero-field values of 3.0, 2.5, 2.2, and 2.0 cm2V−1·sec−1 in close agreement with the polarization-limit Langevin theory." @default.
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- W2018721935 date "1970-12-01" @default.
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- W2018721935 title "Water Cluster Ions: Rates of Formation and Decomposition of Hydrates of the Hydronium Ion" @default.
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- W2018721935 doi "https://doi.org/10.1063/1.1673936" @default.
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