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• W2018738206 abstract "Ceramic composites have been prepared from the system Al2O3ZrO2SiO2 using the sol-gel technique. The influence of catalyst acids and bases on the chemistry, structure, and morphology of the products obtained after heat treatment at various temperatures (800–1400°C) have been studied using powder X-ray diffractometry and transmission electron microscopy. Formation of compounds at higher temperatures have been shown to be related to the various acid-base reactions between the oxides and the catalyst acid or base in the sol. Formation of zircon (ZrSiO4) in the presence of mullite and by direct SiO2ZrO2 reactions in different compositions has been discussed. A new approach based on the molecular electronegativity differences of the component oxides has been made in order to rationalize the observed reactions. Partial charges on oxygen in various oxides have been evaluated using molecular electronegativities and are shown to be consistent both with well-known basicities of component oxides and the observed reactions. The importance of considering electronegativities in oxide reactions is emphasized." @default.
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• W2018738206 date "1990-10-01" @default.
• W2018738206 modified "2023-10-17" @default.
• W2018738206 title "Thermally induced chemical and structural changes in alumina-zirconia-silica gels during the formation of ceramic composites" @default.
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• W2018738206 doi "https://doi.org/10.1016/0022-4596(90)90237-r" @default.
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