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• W2018773357 abstract "We report Raman and infrared absorption spectroscopy along with x-ray diffraction for brucite-type$ensuremath{beta}text{ensuremath{-}}mathrm{Cd}{(mathrm{O}mathrm{H})}_{2}$ to $28phantom{rule{0.3em}{0ex}}mathrm{GPa}$ at $300phantom{rule{0.3em}{0ex}}mathrm{K}$. The OH-stretching modes soften with pressure and disappear at $21phantom{rule{0.3em}{0ex}}mathrm{GPa}$ with their widths increasing rapidly above $5phantom{rule{0.3em}{0ex}}mathrm{GPa}$, consistent with a gradual disordering of the H sublattice at $5--20phantom{rule{0.3em}{0ex}}mathrm{GPa}$ similar to that previously observed for $mathrm{Co}{(mathrm{O}mathrm{H})}_{2}$. Asymmetry in the peak shapes of the OH-stretching modes suggests the existence of diverse disordered sites for H atoms in $mathrm{Cd}{(mathrm{O}mathrm{H})}_{2}$ under pressure. Above $15phantom{rule{0.3em}{0ex}}mathrm{GPa}$, the ${A}_{1g}(T)$ lattice mode shows nonlinear behavior and softens to $21phantom{rule{0.3em}{0ex}}mathrm{GPa}$, at which pressure significant changes are observed: some Raman modes appear, two Raman-active lattice modes and the OH-stretching modes of the low-pressure phase disappear, and the positions of some x-ray diffraction lines change abruptly with the appearance of weak diffraction features. These observations suggest that amorphization of the H sublattice is accompanied by a crystalline-to-crystalline transition at $21phantom{rule{0.3em}{0ex}}mathrm{GPa}$ in $mathrm{Cd}{(mathrm{O}mathrm{H})}_{2}$, which has not been previously observed in the brucite-type hydroxides. The Raman spectra of the high-pressure phase of $mathrm{Cd}{(mathrm{O}mathrm{H})}_{2}$ is similar to those of the high-pressure phase of single-crystal $mathrm{Ca}{(mathrm{O}mathrm{H})}_{2}$ of which structure has been tentatively assigned to the $mathrm{Sr}{(mathrm{O}mathrm{H})}_{2}$ type." @default.
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• W2018773357 title "Vibrational spectroscopy and x-ray diffraction of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mi mathvariant=normal>Cd</mml:mi><mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant=normal>O</mml:mi><mml:mi mathvariant=normal>H</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math>to<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mn>28</mml:mn><mml:mspace width=0.3em…" @default.
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• W2018773357 doi "https://doi.org/10.1103/physrevb.74.024107" @default.
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