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- W2018934866 abstract "Fixed‐energy cross sections, thermal‐translation rate constants, energies of activation, opacity functions, and probabilities of reaction as functions of initial relative orientation angle are presented for the reaction H+H2(v, j)→3H on the lowest‐energy potential surface for selected initial vibrational‐rotational states (v, j) of H2. In agreement with the experimental result for steady dissociation of a thermal mixture of initial states, the collision‐induced dissociation process for these state‐selected processes is found to be considerably enhanced for H as collision partner as compared to Ar as collision partner. We find that the cross sections for collision‐induced dissociation are strongly increasing functions of initial internal energy and initial vibrational quantum number. The general trend at 4500 K is that the rate constants increase more rapidly than the equilibrium populations decreases as we increase v. The activation energies for complete dissociation are larger than the fixed‐state binding energies by 0.2–1.1 eV." @default.
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- W2018934866 date "1983-03-01" @default.
- W2018934866 modified "2023-10-18" @default.
- W2018934866 title "Third body efficiencies for collision‐induced dissociation of diatomics. Rate coefficients for H+H2→3H" @default.
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- W2018934866 doi "https://doi.org/10.1063/1.445040" @default.
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