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• W2018964250 abstract "In this article, we describe a series of new complex salts in which electron-donating cis-{Ru(II)(NH3)(4)}(2+) centers are connected to two electron-accepting N-methyl/aryl-pyridinium groups. These V-shaped complexes contain either monodentate 4,4'-bipyridyl-derived ligands or related chelates based on 2,2':4,4:4',4'''-quaterpyridyl and have been characterized by using various techniques including electronic absorption spectroscopy and cyclic voltammetry. Molecular quadratic nonlinear optical (NLO) responses beta have been determined by using hyper-Rayleigh scattering at 800 nm and also via Stark (electroabsorption) spectroscopic studies on the intense, visible d --> pi metal-to-ligand charge-transfer bands. These experiments reveal that these dipolar pseudo-C(2v)chromophores exhibit two substantial components of the beta tensor, beta(zzz)and beta(zyy), with the difference between them being most marked for the nonchelated systems. Time-dependent density-functional theory and finite field calculations serve to further illuminate the electronic structures and associated linear and NLO properties of the new chromophoric salts." @default.
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• W2018964250 date "2005-03-10" @default.
• W2018964250 modified "2023-10-17" @default.
• W2018964250 title "Syntheses and Properties of Two-Dimensional Charged Nonlinear Optical Chromophores Incorporating Redox-Switchable <i>cis</i>-Tetraammineruthenium(II) Centers" @default.
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• W2018964250 doi "https://doi.org/10.1021/ja0424124" @default.
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