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- W2018998672 abstract "Abstract The self‐assembled boronic ester cavitand capsule 3 quantitatively and tightly encapsulates 2,6‐diacetoxy‐9,10‐bis(arylethynyl)anthracene derivatives 4 a – 4 c as highly fluorescent cruciform guests to form complexes 4 a @ 3 , 4 b @ 3 , and 4 c @( 3 ) 2 . The structural features of capsule 3 , which possesses two polar bowl‐shaped aromatic cavity ends and four large equatorial windows connected by dynamic boronic ester bonds, made it possible to encapsulate cruciform 4 with protection of the reactive anthracene core inside the capsule and with two protruding arylethynyl groups, the π‐conjugated arms of compound 4 , through two of the equatorial windows of the capsule. Thus, complexes 4 a @ 3 , 4 b @ 3 , and 4 c @( 3 ) 2 show greater resistance to photochemical reactions in solution and fluorescence quenching in the powder state compared to free guests 4 . In addition to the improved photostability, restriction of the free rotation of the arylethynyl groups of guests 4 upon encapsulation results in sharpening of the UV/Vis absorption peaks with a red‐shift and a significant increase in some of the two‐photon‐absorption peaks of complexes 4 a @ 3 , 4 b @ 3 , and 4 c @( 3 ) 2 compared with free guests 4 ." @default.
- W2018998672 created "2016-06-24" @default.
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- W2018998672 date "2014-02-25" @default.
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- W2018998672 title "Encapsulation with the Protrusion of Cruciform 9,10-Bis(arylethynyl)anthracene Derivatives in a Self-Assembled Boronic Ester Cavitand Capsule: Photochemical and Photophysical Properties" @default.
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- W2018998672 doi "https://doi.org/10.1002/asia.201400042" @default.
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