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- W2019096718 abstract "A bi-function catalyst containing CuZnAlCr and HZSM-5 was used to generate hydrogen by stream reforming of dimethyl ether (SRD) in a metal foam micro-reactor and a fix-bed reactor. Dimethyl ether conversion of 99% and hydrogen yield of >95% was reached with HZSM-5/CuZnAlCr (mass ratio of 1:1) in the micro-reactor. A suitable balance between the dimethyl ether hydrolysis and methanol reforming steps requires the proper acidity and the metal sites. The CuZnAlCr/HZSM-5 properties, effect of CuZnAlCr to HZSM-5 mass ratio were investigated in the metal foam micro-reactor. Moreover, CO was removed from hydrogen-rich gas by preferential oxidation reaction (CO-PrOx) with PtFe/γ-Al2O3 catalyst in a similar metal foam micro-reactor follows the SRD stage. With the optimized O2/CO ratio and reaction temperature, the CO concentration dropped to <10 ppm and hydrogen yield of ∼90% were achieved in the new-type SRD-COPrOx system. The SRD-COPrOx system provide a constant hydrogen production with CO concentration lower than 10 ppm during 20 h. The results indicate that metal foam micro-reactor has the great potential in the DME steam reforming to supply hydrogen for low-temperature fuel cells." @default.
- W2019096718 created "2016-06-24" @default.
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- W2019096718 date "2014-07-01" @default.
- W2019096718 modified "2023-09-23" @default.
- W2019096718 title "Hydrogen production by steam reforming of dimethyl ether and CO-PrOx in a metal foam micro-reactor" @default.
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- W2019096718 doi "https://doi.org/10.1016/j.ijhydene.2014.04.096" @default.
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