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- W2019169747 abstract "The assumption that the photodissociation of HI proceeds adiabatically is re-examined in the context of recently calculated alignment parameters, a(⟂), for the ground state halogen atoms resulting from photodissociation of the analogous HCl and HBr molecules. The a(⟂) alignment parameters for HCl, HBr, and HI are determined from time-dependent quantum mechanical wave packet calculations based on the best available ab initio electronic structure for each molecule. The experimental measurement of the alignment of the I(2P3/2) atoms is proposed as a stringent test of whether the photodissociation is adiabatic or involves non-adiabatic coupling of the A1Π1 and a3Π1 electronic states. © 2007 Wiley Periodicals, Inc. Int J Quantum Chem, 2007" @default.
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- W2019169747 date "2007-01-01" @default.
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- W2019169747 title "The photodissociation of hydrogen iodide: Is it adiabatic?" @default.
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- W2019169747 doi "https://doi.org/10.1002/qua.21414" @default.
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