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- W2019197706 abstract "The adsorption of four fullerene derivatives, including Re(C60Me5)(CO)3, Ru(C60Ph5)Cp, C60(C6H4C6H4−COOH)5Me, and C60(C6H4−CC−SiMe2C12H25)5Me, on a Au(111) surface has been investigated by scanning tunneling microscopy (STM) and cyclic voltammetry. High-resolution STM images reveal that Re(C60Me5)(CO)3 forms a well-ordered (2√3 × 2√3)R30° structure. Different from C60 on Au(111), the so-called “in-phase” structure is not found with the attachment of methyl and Re(CO)3 groups. With the increase of substituent size, disordered adlayers have been observed for Ru(C60Ph5)Cp and C60(C6H4C6H4−COOH)5Me. However, the individual molecules could be distinguished in STM images, suggesting that the two molecules interact strongly with the Au(111) surface. When the substituent size is further increased, a multilayered structure is formed for C60(C6H4−CC−SiMe2C12H25)5Me. This is because of molecular aggregation in the bulk solution, which occurs at very low concentration. These results indicate that the structures of fullerene derivatives play an essential role in adlayer formation through adjusting molecule−substrate and molecule−molecule interactions." @default.
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- W2019197706 date "2010-02-01" @default.
- W2019197706 modified "2023-10-03" @default.
- W2019197706 title "Substituent-Dependent Ordering of Adlayer Structures of Fullerene Derivatives Adsorbed on Au(111): A Scanning Tunneling Microscopy Study" @default.
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- W2019197706 doi "https://doi.org/10.1021/jp9114173" @default.
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