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- W2019295943 abstract "Abstract Absorption spectrum of a transient species of Pu(VII), [PuO 2 (CO 3 ) 2 (OH) 2 ] 3- , has been obtained in the flash photolysis of solutions containing (50–500) x 10 -6 mol dm -3 Pu(VI) and (5–30) x 10 -3 mol dm -3 Na 2 CO 3 at pH 12.5. The transient species appears to form through the reaction of CO - 3 ion radical with [PuO 2 (CO 3 )(OH) 2 ] 2- [k = (1.45 +- 0.06) x 10 7 mol -1 dm 3 s -1 ] and decays spontaneously with a rate constant of (7.61 +- 0.09) x 10 2 s -1 . Evidence for the photoreduction of Pu(VI) has also been obtained and a reaction mechanism is proposed to explain the results." @default.
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- W2019295943 date "1986-01-01" @default.
- W2019295943 modified "2023-09-26" @default.
- W2019295943 title "Flash photolytic investigations on the reaction between Pu(VI) and CO-3 in alkaline medium" @default.
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