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- W2019455422 abstract "The zeroth and second spectral moments for the far infrared spectral intensity of a polar liquid are analyzed from first principles, taking into account the first-order dipole–induced dipole contribution. The results, based on evaluating the equilibrium averages of appropriate correlation functions, are simplified by considering that the liquid pair distribution function can be approximated by a truncated expansion in terms of Wigner rotation functions. Averages involving three- and four-molecule distribution functions are not considered in the present calculation. The calculated zeroth moment for acetonitrile, M(0)=17.5 D2, compares favorably with the experimental value of 20.7 D2. The difference probably reflects the neglect of three- and four-molecule terms as well as higher order induction effects." @default.
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- W2019455422 date "1990-12-01" @default.
- W2019455422 modified "2023-09-24" @default.
- W2019455422 title "Interaction induced contributions to the far infrared spectrum of a polar fluid: Zeroth and second spectral moments" @default.
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- W2019455422 doi "https://doi.org/10.1063/1.459387" @default.
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