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• W2019502743 abstract "Esperamicin A1 effectively breaks DNA strands upon heating at 50 degrees C. The preferential DNA cutting sites of heat-activated esperamicin A1 are random and clearly differ from those of thiol- or UV-light-mediated DNA breakage with esperamicin A1. The absence of heat-induced DNA cleavage by esperamicin Z and the induction of the DNA breakage by esperamicin A1 disulfide indicate that (1) the enediyne core plays a significant role in this DNA strand scission and (2) the DNA cutting with the heat-activated esperamicin antibiotics does not necessarily require a trisulfide trigger in the aglycon portion. On the basis of the present results, a probable mechanism for the heat-induced DNA cleavage of esperamicin A1 has been proposed." @default.
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• W2019502743 date "1991-09-01" @default.
• W2019502743 modified "2023-10-16" @default.
• W2019502743 title "Heat-induced DNA cleavage by esperamicin antitumor antibiotics" @default.
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• W2019502743 doi "https://doi.org/10.1021/bi00102a016" @default.
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