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- W2019686211 endingPage "611" @default.
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- W2019686211 abstract "A cationic CpRu complex of chiral picolinic acid derivatives [(R)- or (S)-Cl-Naph-PyCOOCH2CH═CH2] catalyzes asymmetric intramolecular dehydrative N-allylation of N-substituted ω-amino- and -aminocarbonyl allylic alcohols with a substrate/catalyst ratio of up to 2000 to give α-alkenyl pyrrolidine-, piperidine-, and azepane-type N-heterocycles with an enantiomer ratio of up to >99:1. The wide range of applicable N-substitutions, including Boc, Cbz, Ac, Bz, acryloyl, crotonoyl, formyl, and Ts, significantly facilitates further manipulation toward natural product synthesis." @default.
- W2019686211 created "2016-06-24" @default.
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- W2019686211 date "2011-12-23" @default.
- W2019686211 modified "2023-10-17" @default.
- W2019686211 title "Enantioselective Synthesis of Pyrrolidine-, Piperidine-, and Azepane-Type <i>N</i>-Heterocycles with α-Alkenyl Substitution: The CpRu-Catalyzed Dehydrative Intramolecular <i>N</i>-Allylation Approach" @default.
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- W2019686211 doi "https://doi.org/10.1021/ol203218d" @default.
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