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- W2019688606 abstract "The ground-state rotational spectra of 24 isotopomers of ethynylstannane have been observed by pulsed-jet, Fourier-transform microwave spectroscopy. The spectroscopic constants, B0,DJ and DJK are reported for symmetric-top isotopomers H3nSn12C12CH, where n = 116, 117, 118, 119, 120, 122 and 124, D3nSn12C12CH, where n = 116, 118, 120, 122 and 124, H3nSn13C12 CH and H3nSn12C13CH , where n = 116,118 and 120, and H3nSn12C12CD, where n = 116, 118 and 120. In addition, the values of A0, B0, C0, ΔJ and ΔJK were obtained for the three asymmetric-top isotopomers DH2nSn12C12CH, where n = 116, 118 and 120. Hyperfine structure was resolved and assigned in the transitions of the isotopomers H3nSnCCD, where n = 116, 118 and 120, and in the isotopomers H3117SnCCH and H3119SnCCH. In the former group, the hyperfine structure arises from D nuclear quadrupole coupling while in the latter group its origin lies in the spin-rotation coupling of the I = 1/2 Sn nuclear spin to the rotational motion. For these isotopomers, D nuclear quadrupole and spin-rotation coupling constants are determined where appropriate. The rotational constants obtained for the 24 isotopomers of H3SnCCH were used to obtain the following types of molecular geometry for ethynylstannane: r0, rs, and rm." @default.
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- W2019688606 date "2006-01-01" @default.
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- W2019688606 title "The ground-state rotational spectrum and molecular geometry of ethynylstannane" @default.
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- W2019688606 doi "https://doi.org/10.1039/b517507k" @default.
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