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• W2019796508 abstract "We have examined the photochemical reactions occurring after irradiation at 200 nm of the aqueous nitrate ion, NO3(-)(aq). Using femtosecond transient absorption spectroscopy over the range 194-388 nm, we have characterized the formation and subsequent relaxation of the primary photoproducts of nitrate photolysis. The dominant photoproduct is the cis-isomer of peroxynitrite, which accounts for 48% of the excited state molecules initially produced. A slightly smaller fraction, 44%, of the excited molecules return to the electronic ground state of NO3(-) and relax to the vibrational ground state in 2 ps. The remaining 8% of the molecules initially excited react via the *NO + *O2(-) or the NO- + O2 dissociation channels. Formation of NO2(-) and *NO2 is not observed, suggesting that the previous observations of these species in steady-state photolysis are caused by reactions occurring on a longer time scale." @default.
• W2019796508 created "2016-06-24" @default.
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• W2019796508 date "2003-11-18" @default.
• W2019796508 modified "2023-10-06" @default.
• W2019796508 title "The Primary Photodynamics of Aqueous Nitrate: Formation of Peroxynitrite" @default.
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• W2019796508 doi "https://doi.org/10.1021/ja030135f" @default.
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