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• W2019807780 endingPage "660" @default.
• W2019807780 startingPage "653" @default.
• W2019807780 abstract "The synthesis and characterization of two isoreticular metal-organic frameworks (MOFs), {[Cd(bdc)(4-bpmh)]}n⋅2 n(H2O) (1) and {[Cd(2-NH2bdc)(4-bpmh)]}n⋅2 n(H2O) (2) [bdc = benzene dicarboxylic acid; 2-NH2bdc = 2-amino benzene dicarboxylic acid; 4-bpmh = N,N-bis-pyridin-4-ylmethylene-hydrazine], are reported. Both compounds possess similar two-fold interpenetrated 3D frameworks bridged by dicarboxylates and a 4-bpmh linker. The 2D Cd-dicarboxylate layers are extended along the a-axis to form distorted square grids which are further pillared by 4-bpmh linkers to result in a 3D pillared-bilayer interpenetrated framework. Gas adsorption studies demonstrate that the amino-functionalized MOF 2 shows high selectivity for CO2 (8.4 wt % 273 K and 7.0 wt % 298 K) over CH4 , and the uptake amounts are almost double that of non-functional MOF 1. Iodine (I2 ) adsorption studies reveal that amino-functionalized MOF 2 exhibits a faster I2 adsorption rate and controlled delivery of I2 over the non-functionalized homolog 1." @default.
• W2019807780 created "2016-06-24" @default.
• W2019807780 creator A5030031955 @default.
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• W2019807780 creator A5070299271 @default.
• W2019807780 date "2014-12-18" @default.
• W2019807780 modified "2023-10-13" @default.
• W2019807780 title "Tuning CO₂Uptake and Reversible Iodine Adsorption in Two Isoreticular MOFs through Ligand Functionalization" @default.
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• W2019807780 doi "https://doi.org/10.1002/asia.201403123" @default.
• W2019807780 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25523149" @default.
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