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- W2019812693 abstract "Abstract The Ce 1− x R x Ni 2.5 Cu 2.5 (R = La,Pr; 0.8 ⩾ x ⩾ 0.3) and PrNi 5− x M x (M = Cu, Fe; 0.5 ⩾ x ⩾ 2.5) alloys were investigated for their hydriding characteristics in the temperature range 0–70°C and hydrogen pressure range 0.01–50 atm. The nonlinear behaviour of unit cell volume vs x in Ce 1– x La x Ni 2.5 Cu 2.5 suggests that both size and electronic effects are involved. The partial replacement of Ce by La and Ni by Cu in CeNi 5 causes a substantial reduction in the hydrogen sorption pressures without significantly impairing its hydrogen capacity. It was observed that Fe is more effective than Cu in stabilizing PrNi 5 -H 2 . The high values of the molar entropy of hydrogen of the β-hydrides studied, S β H , are attributed to extensive hydrogen disorder in the interstitial sites of the host lattice. A linear correlation between the hydride decomposition pressures (or free energy) and the unit cell volume. V c , of the host alloys was observed. This behavior is helpful in predicting the stabilities of new hydrides in a given substitutional alloy series." @default.
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- W2019812693 date "1986-01-01" @default.
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- W2019812693 title "Stability of some ternary and quaternary CeNi5-based and PrNi5-based hydride systems☆" @default.
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