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• W2019820797 endingPage "074715" @default.
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• W2019820797 abstract "We study the X-ray magnetic circular dichroism (XMCD) spectra at the U M 4,5 and N 4,5 edges of uranium monochalcogenides, U X where X =S, Se, and Te, examining the applicability of the XMCD sum rules to U X by the fully relativistic full-potential linear-combination-of-atomic-orbitals (LCAO) method based on the density functional theory. To extract the transitions relevant to the sum-rule analysis, we employ the Mulliken population analysis (MPA). Using the MPA, the orbital sum rule is found to be valid to 10–20% for the M 4,5 edges and valid to 5–15% for the N 4,5 edges. On the other hand, the spin sum rule is found to be valid to 10–20% for the M 4,5 edges whereas valid to 30–35% for the N 4,5 edges. Furthermore, it is found that the calculated XMCD spectra are consistent with a recent experimental observation that the intensity of the N 4,5 XMCD signal is comparable to that of the M 4,5 XMCD signal although contradicting a previous theoretical prediction that the XMCD intensity at the N 4,5 edges is one order of magnitude smaller than that at the M 4,5 edges." @default.
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• W2019820797 date "2009-07-15" @default.
• W2019820797 modified "2023-09-23" @default.
• W2019820797 title "Mulliken Population Analysis of X-ray Magnetic Circular Dichroism in Uranium Monochalcogenides: Examination of Sum Rules by Fully Relativistic Full-Potential LCAO Method" @default.
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• W2019820797 doi "https://doi.org/10.1143/jpsj.78.074715" @default.
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