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- W2019890210 abstract "Results are presented of calculations on the experimentally observed lifetime enhancement of high principal quantum number nf(N+=2) and np(N+=0) Rydberg states of the NO molecule in small dc electric fields. A Hund’s case (d) molecular Hamiltonian is introduced, which describes intramolecular interactions between low angular momentum Rydberg states as a result of core penetration and l mixing caused by the electric field. Eigenstates of the molecule in the electric field are obtained by diagonalization of the Hamiltonian and an effective decay time is determined which describes the multiexponential decay of the superposition of (Stark) states which is excited experimentally. The calculations reproduce the striking onset of the lifetime enhancement of the np(N+=0) series, which was observed experimentally. Both for the nf(N+=2) and np(N+=0) Rydberg series, core penetration by low-l states leads to extensive interseries coupling for several values of the principal quantum number." @default.
- W2019890210 created "2016-06-24" @default.
- W2019890210 creator A5021608732 @default.
- W2019890210 date "1996-11-01" @default.
- W2019890210 modified "2023-10-16" @default.
- W2019890210 title "Lifetimes of Rydberg states in ZEKE experiments. III. Calculations of the dc electric field dependence of predissociation lifetimes of NO" @default.
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- W2019890210 doi "https://doi.org/10.1063/1.472592" @default.
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