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• W2019901604 abstract "Derivatives of quinolinium iodide have been found to exhibit second-order nonlinear optical (NLO) response in their crystalline form. The quaternary amine functionality is introduced as an electron-withdrawing group in NLO-active chromophores. While their electron-accepting capabilities are somewhat weaker than those of the nitro group, these organic salts show a much more favorable transparency−nonlinearity tradeoff for blue second harmonic generation (SHG) NLO applications. Here we present crystal growth and characterization via X-ray diffraction (XRD), NMR, FTIR, and optical spectroscopy measurements. Experimental linear optical features are fully consistent with INDO/SCI−SOS theoretical calculations. These latter provide a rationale for the NLO response of these materials. Calculations predict a sizable molecular nonlinearity, which parallels the wavelength of the lowest charge-transfer transition. In addition, a direct correlation between SHG powder response to the β crystallographic angle is observed." @default.
• W2019901604 created "2016-06-24" @default.
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• W2019901604 date "1999-09-29" @default.
• W2019901604 modified "2023-10-03" @default.
• W2019901604 title "Quinolinium-Derived Acentric Crystals for Second-Order NLO Applications with Transparency in the Blue" @default.
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• W2019901604 doi "https://doi.org/10.1021/jp991616h" @default.
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