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- W2019907360 abstract "We present a new scheme for performing optical spectroscopy on single molecules. A glass capillary with a diameter of 600 nm filled with an organic crystal tightly guides the excitation light and provides a maximum spontaneous emission coupling factor ($beta$) of 18% for the dye molecules doped in the organic crystal. Combination of extinction, fluorescence excitation and resonance fluorescence spectroscopy with microscopy provides high-resolution spatio-spectral access to a very large number of single molecules in a linear geometry. We discuss strategies for exploring a range of quantum optical phenomena, including coherent cooperative interactions in a mesoscopic ensemble of molecules mediated by a single mode of propagating photons." @default.
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- W2019907360 date "2014-11-18" @default.
- W2019907360 modified "2023-09-24" @default.
- W2019907360 title "Coherent Interaction of Light and Single Molecules in a Dielectric Nanoguide" @default.
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- W2019907360 doi "https://doi.org/10.1103/physrevlett.113.213601" @default.
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