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- W2019910404 abstract "The graph theoretical/algebraic λ-model has been applied to describe catalyzed [2 + 2] cycloadditions. Based upon a logical analysis of the individual steps in the catalytic reactions (adsorption, catalytic bond rearrangement, desorption), graphs describing reactants, intermediates and products have been derived. The continuous character of the whole process has been described by an ensemble of all possible structural mixtures of the graphs involved using so-called reaction parameters λi. By the assumption of mechanisms most commonly discussed in the literature, certain reductions in this ensemble may be introduced. By solving the corresponding eigenvalue problems, correlation diagrams have been derived which lead, in particular, to selection rules regarding the course of catalyzed [2 + 2] cycloadditions." @default.
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- W2019910404 date "1985-03-01" @default.
- W2019910404 modified "2023-09-25" @default.
- W2019910404 title "Graph theoretical modelling of environmental influences in catalytic [2 + 2] cycloadditions" @default.
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- W2019910404 doi "https://doi.org/10.1016/0304-5102(85)87004-8" @default.
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