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• W2019918269 abstract "Abstract Single-walled carbon nanotubes (SWNTs) were oxidatively treated to introduce carboxyl groups on the carbon nanotube (CNT) surfaces. The carboxylated CNTs (CNT-COOHs) were incorporated into a redox hydrogel film made from a copolymer of polyacrylamide (PAA) and poly (N-vinylimidazole) (PVI) complexed with [Os(4,4′-dichloro-2,2′-bipyridine) 2 Cl] +/2+ (PAA-PVI-[Os(dCl-bpy) 2 Cl] +/2+ ) wiring bilirubin oxidase (BOD) enzyme molecules. The constructed BOD cathode was employed for the electrocatalytic O 2 reduction. The performance was compared with that of the BOD cathode without the incorporation of CNT-COOHs. At an electrode rotating with a 500 rpm speed in an air-saturated 0.15 M NaCl buffer at pH 7.4, an enhancement of the O 2 reduction current density from 0.24 mA/cm 2 to 0.51 mA/cm 2 after the CNT incorporation was observed. The BOD cathode containing CNT-COOHs showed less decay against halide ion inhibitions. For the BOD cathode with no CNT-COOHs incorporated, the current decreased by 22% with 0.9 M NaCl added, and 27% with 0.9 M KBr added, but, with CNT-COOHs incorporated, only 6% and 5% current decays were measured, respectively. Finally, the constructed BOD cathode with CNT-COOHs incorporated showed better stability. When a potential of 0.1 V vs. Ag/AgCl was applied to the cathode being rotated with a speed of 200 rpm for 8000 s, almost no current decay was measured, while 7% current decay was measured for the BOD cathode with no CNT-COOHs incorporated." @default.
• W2019918269 created "2016-06-24" @default.
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• W2019918269 date "2014-01-01" @default.
• W2019918269 modified "2023-09-26" @default.
• W2019918269 title "Enhanced performance of the wired-bilirubin oxidase oxygen cathode with incorporation of carboxylated single-walled carbon nanotubes" @default.
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• W2019918269 doi "https://doi.org/10.1016/j.electacta.2013.10.213" @default.
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