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- W2019924983 abstract "Experimental quartz solubilities in H2O (Anderson and Burnham, 1965, 1967) were used together with equations of state for quartz and aqueous species (Helgesonet al., 1978; Walther and Helgeson, 1977) to calculate the dielectric constant of H2O (ϵH2O) at pressures and temperatures greater than those for which experimental measurements (Heger, 1969; Lukashovet al., 1975) are available (0.001 ⩽ P ⩽ 5 kb and 0 ⩽ T ⩽ 600°C). Estimates of ϵH2O computed in this way for 2 kb (which are the most reliable) range from 9.6 at 600°C to 5.6 at 800°C. These values are 0.5 and 0.8 units greater, respectively, than corresponding values estimated by Quist and Marshall (1965), but they differ by <0.3 units from extrapolated values computed from Pitzer's (1983) adaptation of the Kirkwood (1939) equation. The estimates of ϵH2O generated from quartz solubilities at 2 kb were fit with a power function of temperature, which was then used together with equations and data given by Helgeson and Kirkham (1974a,b, 1976) Helgesonet al. (1981), and Helgeson (1982b, 1984) to calculate Born functions, Debye Hückel parameters, and the thermodynamic properties of Na+, K+, Mg++, Ca++, and other aqueous species of geologic interest at temperatures to 900°C." @default.
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- W2019924983 date "1984-11-01" @default.
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- W2019924983 title "Estimation of the dielectric constant of H2O from experimental solubilities of quartz, and calculation of the thermodynamic properties of aqueous species to 900°C at 2 kb" @default.
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