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- W2019931259 abstract "Heterogeneous perturbations 2 E + ~ 2 Π of largely different magnitudes are observed with high resolution in the vacuum-ultraviolet absorption and in the infrared emission spectrum of the NO molecule. The rotational interactions between 2 Σ + Rydberg states and levels of the B 2 Π non-Rydberg state are shown to be configurationally forbidden, but produced by the configuration interaction between the non-Rydberg levels and 2 Π Rydberg states. The latter together with the 2 Σ + Rydberg states form p complexes. In this way the interactions display the l uncoupling in the complexes; they can be evaluated theoretically and can be analyzed fully. The cases of the strong interactions D 2 Σ + (v = 3) ~ B 2 Π(v = 16)and D 2 Σ + (v = 5) ~ B 2 Π(v = 21) and of the weaker D 2 Σ + (v = 1) ~ B 2 Π(v = 11), all three observed as perturbations in ε bands crossing 3 bands, are discussed in detail. It is further shown that perturbations between γ bands and β bands as well as perturbations between analogous bands of higher principal quantum number are absent, and thus the assignment of the A 2 Σ + and E 2 Σ + states to the s Rydberg series is confirmed." @default.
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- W2019931259 date "1968-04-15" @default.
- W2019931259 modified "2023-09-27" @default.
- W2019931259 title "Absorption spectrum of the NO molecule. VIII. The heterogeneous (<sup>2</sup>Σ–<sup>2</sup>Π) interactions between excited states" @default.
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- W2019931259 doi "https://doi.org/10.1139/p68-126" @default.
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