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• W2019957698 abstract "It is shown that the atom-molecule collision problem in the presence of an external electric field can be solved using the total angular momentum representation in the body-fixed coordinate frame, leading to a computationally efficient method for ab initio modeling of low-temperature scattering phenomena. Our calculations demonstrate rapid convergence of the cross sections for vibrational and Stark relaxation in He-CaD collisions with the number of total angular momentum states in the basis set, leading to a 5- to 100-fold increase in computational efficiency over the previously used methods based on the fully uncoupled space-fixed representation. These results open up the possibility of carrying out numerically converged quantum scattering calculations on a wide array of atom-molecule collisions and chemical reactions in the presence of electric fields." @default.
• W2019957698 created "2016-06-24" @default.
• W2019957698 creator A5081725229 @default.
• W2019957698 date "2012-05-22" @default.
• W2019957698 modified "2023-09-27" @default.
• W2019957698 title "Total-angular-momentum representation for atom-molecule collisions in electric fields" @default.
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• W2019957698 doi "https://doi.org/10.1103/physreva.85.052710" @default.
• W2019957698 hasPublicationYear "2012" @default.
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