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- W2019968015 abstract "A systematic sum frequency generation vibrational spectroscopy study is conducted on the gas−liquid interface of room-temperature ionic liquids. The compounds contain ammonium and pyrrolidinium based cations, to which alkyl substituents of different length and/or functional groups are attached, and they are all combined with the bis-trifluoromethanesulfonimide anion ([imide]-). The alkyl chain length shows a strong effect on the ordering of the chains at the topmost layer, reaching the maximum order for (C4H9)N+(CH3)2(C3H7) and (C6H13)N+C4H8(CH3). There is also evidence of gauche defects for longer alkyl chains, and changes in the spectral features for the shortest ones. The substitution of a carbon atom in the chain by oxygen, and its per-deuteration, provides the means to acquire a more complete description of the surface structure, and an unambiguous assignment of the vibrations detected in the SFG spectra. Finally, a brief comparison between alkylpyrrolidinium, and previously studied alkylimidazolium, cations is also established." @default.
- W2019968015 created "2016-06-24" @default.
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- W2019968015 date "2008-01-18" @default.
- W2019968015 modified "2023-10-15" @default.
- W2019968015 title "Sum Frequency Generation Studies of Ammonium and Pyrrolidinium Ionic Liquids Based on the Bis-trifluoromethanesulfonimide Anion" @default.
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- W2019968015 doi "https://doi.org/10.1021/jp077008g" @default.
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