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- W2019970724 abstract "Intramolecular photoinduced charge separation and recombination within the donor−acceptor molecule 4-(N-pyrrolidino)naphthalene-1,8-imide-pyromellitimide, 5ANI−PI, are studied using ultrafast transient absorption spectroscopy in the room-temperature ionic liquid, 1-ethyl-3-methylimidazolium bis(trifluoromethanesulfonyl)amide [EMIM][Tf2N]. The rate constants of both photoinduced charge separation and charge recombination for 5ANI−PI in [EMIM][Tf2N] are comparable to those observed in pyridine, which has a static dielectric constant similar to that of [EMIM][Tf2N] but a viscosity that is nearly 2 orders of magnitude lower than that of [EMIM][Tf2N]. The electron-transfer dynamics of 5ANI−PI in [EMIM][Tf2N] are compared to those in pyridine as a function of temperature and are discussed in the context of recently reported ionic liquid solvation studies." @default.
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- W2019970724 date "2007-09-18" @default.
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- W2019970724 title "Intramolecular Electron Transfer within a Covalent, Fixed-Distance Donor−Acceptor Molecule in an Ionic Liquid" @default.
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- W2019970724 doi "https://doi.org/10.1021/jp075567h" @default.
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