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- W2020127129 abstract "Reactions of [RuCl2L4] (L = PMe3, PMe2Ph or PMePh2) with 2-lithiomethyl-1-methylnaphthalene or 2-lithiomethyl-3-methylnaphthalene lead to [Ru(CH2C10H6CH2)L3] which contain coordinated 1,2- or 2,3-naphthoquinodimethane moieties. Spectroscopic studies confirm these formulations and suggest significant localization of the double bonds, at least for the 1,2-naphthoquinodimethane fragment. For L = PMe3 and 2-lithiomethyl-1-methylnaphthalene formation of the 1,2-naphthoquinodimethane complex is accompanied by the formation of [Ru(CH2C10H6CH2)(PMe3)4] in which the organic moiety acts as a dialkyl, two-electron donor. Surprisingly for L = PMe2Ph and 2-lithiomethyl-3-methylnaphthalene, the naphthoquinodimethane is not formed but the major product, although not isolated in a pure state, appears to be [Ru(CH2C6H10CH3)Cl(PMe2Ph)3] in which the organic group is coordinated in an η3 (allyl) mode. Plausible mechanisms, which account for the various products formed in these reactions are presented." @default.
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- W2020127129 date "1988-01-01" @default.
- W2020127129 modified "2023-09-26" @default.
- W2020127129 title "Naphthoquinodimethane complexes of ruthenium(O)" @default.
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- W2020127129 doi "https://doi.org/10.1016/s0277-5387(00)80709-3" @default.
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