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- W2020155940 abstract "Electron transfer at the molecule−metal interface of self-assembled monolayers of 1,1‘;4‘,1‘ ‘-terphenyl-4‘ ‘-thiol (BBB) and its partially fluorinated counterpart (BFF: p-thiophenyl-nonafluorobiphenyl) on Au(111) is investigated by core-hole clock spectroscopy. Ultrafast electron transfer at the BBB/Au(111) interface in the low-femtosecond regime (on the same time scale as the C 1s core-hole lifetime, ∼6 fs) was observed. In contrast, for BFF/Au(111), the interface electron transfer was forbidden during the core-hole decay. This strongly suggests that fluorination of phenyl rings significantly enhances the localization of the excited electrons in the LUMO." @default.
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- W2020155940 date "2005-12-31" @default.
- W2020155940 modified "2023-10-07" @default.
- W2020155940 title "Effect of Functional Group (Fluorine) of Aromatic Thiols on Electron Transfer at the Molecule−Metal Interface" @default.
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- W2020155940 doi "https://doi.org/10.1021/ja056324a" @default.
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