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• W2020180493 abstract "Theoretical expressions for photocurrents at p-type and n-type semiconductors have been set up under the initial assumption that the rate determining step is the discharge process for H3O+ at p-type electrode and OH− (or H2O) at n-type electrode. The photocurrents at individual electrodes are calculated by using the characteristics of semiconductor electrodes, e.g. energy gap etc. The calculated results for the quantum efficiencies are from 10−2 to 10% depending on the properties of the semiconductors (c.f. a maximum of 0.1% in the metal case). The theoretical results for TiO2 are inconsistent with observations. Consequently, the presence of surface states and the supply of holes as the rate determining step are introduced into the model's formalism and yield results consistent with observation. The photocurrents or whole cells are calculated, and finally the hydrogen production rate under solar irradiation is evaluated for a typical cell." @default.
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• W2020180493 date "1977-01-01" @default.
• W2020180493 modified "2023-10-11" @default.
• W2020180493 title "Theoretical treatment of the photoelectrochemical production of hydrogen" @default.
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• W2020180493 doi "https://doi.org/10.1016/0360-3199(77)90004-0" @default.
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