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- W2020202470 abstract "Redistribution and depolarisation of light scattered by atoms undergoing collisions outside the impact region of the line profile has been studied experimentally and theoretically. In a cell experiment intensity and linear degree of polarisation of the fluorescence components 3 2 S 1/2 to or from 3 2 P 1/2,3/2 of Na atoms induced by collisions with Ar buffer gas atoms were measured as functions of the laser frequency omega L . The decrease of polarisation of the D 2 component observed when omega L is shifted away from the D 2 toward D 1 resonance disagrees with calculations on the basis of the factorisation approximation of the theory of redistribution. Using Baylis (1975) potentials for the Na/Ar system, the effect is interpreted in terms of adiabatic coupling of the 3 2 P 3/2 electronic angular momentum to the collision axis during 'strong' collisions, giving rise to a greater than average depolarisation." @default.
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- W2020202470 title "Far wing depolarisation of collision-induced fluorescence" @default.
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